DAPG biocontrol sensor (PhlF + CRISPRi)

Detects 2,4-diacetylphloroglucinol (DAPG), an antibiotic made by biocontrol pseudomonads in soil. The Marionette PhlF sensor gates a CRISPRi circuit driving a visible pigment, in the soil chassis P. putida KT2440 — useful for monitoring soil biocontrol activity.

Chemical / metaboliteBSL-1 chassistemplateDAPGbiocontrolantibioticsoilagriculturechemicalMarionetteCRISPRi
Input
2,4-Diacetylphloroglucinol (DAPG)
Chemical / metabolite
Sense
CRISPRi-repression
dCas9 (S. pyogenes, catalytically dead)
Chassis
Pseudomonas putida KT2440
BSL-1
Output
amilCP
pigment

What it detects

Analyte
2,4-Diacetylphloroglucinol (DAPG) — PhlF responds across µM DAPG
Category
Chemical / metabolite
Signal
DAPG, an antifungal antibiotic produced by biocontrol Pseudomonas in the rhizosphere

Genetic circuit

⤢ click to enlarge

Genetic construct (SBOL)

The DNA construct as transcription units, drawn with SBOL Visual part glyphs.

⤢ click to enlarge

CRISPR sensing mechanism

Strategy
CRISPRi-repression · NOT logic
Cas protein
dCas9 (S. pyogenes, catalytically dead)
Analyte sensor
PhlF de-represses its promoter on binding DAPG.
Signal flow
DAPG -> PhlF releases PphlF -> transcribes an anti-pigment sgRNA -> CRISPRi represses a constitutive amilCP cassette -> pigment fades with DAPG (NOT). Pair an inverter for colour-on.

Safe chassis

Pseudomonas putida KT2440Pseudomonas putida

A certified safety-strain soil bacterium with exceptional solvent/stress tolerance and diverse metabolism. The premier chassis for environmental biosensing of pollutants and heavy metals in soil and water.

BSL-1

Genetic parts

PartRoleSource / id
PhlF regulator
DAPG-responsive repressor; a widely used orthogonal regulator.
regulatorMarionette sensor (Meyer et al. 2019); Pseudomonas phl system
PphlF promoter
De-repressed by DAPG-bound PhlF.
promoterphl operon promoter
Anti-pigment sgRNAsgRNAdesigned against the amilCP promoter
sgRNA scaffold (SpCas9)
GTTTTAGAGCTAGAAATAGCAAGTTAAAATAAGGCTAGTCCGTTATCAACTTGAAAAAGTGGCACCGAGTCGGTGC
sgRNAStandard SpCas9 scaffold
dCas9dCas9CRISPRi (established in P. putida)
amilCP chromoproteinreporterBBa_K592009

Output & readout

Type
pigment
Reporter
amilCP
Readout
Visible pigment (naked eye / smartphone)
Positive result
Pigment change reports soil DAPG (biocontrol activity).

Performance

Limit of detection
PhlF Marionette sensor: µM DAPG (module-validated).
Dynamic range
~1-100 µM DAPG
Response time
~180 min
Device validated
No — design template (parts validated individually)

PhlF is a characterised orthogonal Marionette repressor; integrated CRISPRi device is a design template.

Safety

Biosafety level
BSL-1 (non-pathogenic chassis)
GRAS chassis
No
Biocontainment
P. putida KT2440 certified HV1 safety host; add containment for field use.
Field-deployable
Yes (with containment)

Soil chassis suited to rhizosphere monitoring; instrument-free readout.

Build & run

#StageStep
1designDesign anti-pigment sgRNA
Target the amilCP promoter; check host off-targets.
2assemblyAssemble units
TU1: PhlF + PphlF -> sgRNA. TU2: dCas9 + constitutive amilCP. SEVA vectors.
3transformationTransform P. putida KT2440
Electroporate; select; confirm baseline pigment without DAPG.
4inductionExpose to sample
Add soil eluate + DAPG standard curve.
5readoutScore colour
Compare pigment to the curve.

Source & parts

Design
Design template combining the Marionette PhlF DAPG sensor with P. putida CRISPRi
Parts validated in
  • Meyer et al. 2019, Nat. Chem. Biol. (Marionette sensors, PhlF)
  • Qi et al. 2013, Cell (CRISPRi)
License
Parts per their original sources; design template CC BY 4.0