Choline sensor (BetI + CRISPRi)

Detects choline, a dietary precursor of the cardiovascular-risk metabolite TMA/TMAO in the gut. The Marionette BetI sensor gates a CRISPRi circuit driving a fluorescent reporter, in the probiotic E. coli Nissle 1917.

Clinical / gut biomarkerBSL-1 chassistemplatecholineTMAOmetaboliteclinical-gutprobioticNissleMarionetteCRISPRi
Input
Choline
Clinical / gut biomarker
Sense
CRISPRi-repression
dCas9 (S. pyogenes, catalytically dead)
Chassis
E. coli Nissle 1917
BSL-1
Output
sfGFP
fluorescent

What it detects

Analyte
Choline — BetI responds across µM-mM choline
Category
Clinical / gut biomarker
Signal
Luminal choline, the dietary precursor of gut-microbial TMA (and host TMAO)

Genetic circuit

⤢ click to enlarge

Genetic construct (SBOL)

The DNA construct as transcription units, drawn with SBOL Visual part glyphs.

⤢ click to enlarge

CRISPR sensing mechanism

Strategy
CRISPRi-repression · NOT logic
Cas protein
dCas9 (S. pyogenes, catalytically dead)
Analyte sensor
BetI de-represses the Pbet promoter on binding choline.
Signal flow
Choline -> BetI releases Pbet -> transcribes an anti-reporter sgRNA -> CRISPRi inverts a constitutive reporter (NOT). Pair an inverter for turn-on monitoring of dietary choline load.

Safe chassis

E. coli Nissle 1917Escherichia coli

A probiotic E. coli used in humans for over a century (Mutaflor). Colonizes the gut safely, making it the chassis of choice for clinical / gut biomarker biosensors.

BSL-1probiotic

Genetic parts

PartRoleSource / id
BetI regulator
Choline-responsive repressor.
regulatorMarionette sensor (Meyer et al. 2019); E. coli bet system
Pbet promoter
De-repressed by choline-bound BetI.
promoterE. coli betIBA promoter
Anti-reporter sgRNAsgRNAdesigned against the reporter promoter
sgRNA scaffold (SpCas9)
GTTTTAGAGCTAGAAATAGCAAGTTAAAATAAGGCTAGTCCGTTATCAACTTGAAAAAGTGGCACCGAGTCGGTGC
sgRNAStandard SpCas9 scaffold
dCas9dCas9Qi et al. 2013 (CRISPRi)
sfGFP reporter
Recoverable from stool for non-invasive readout.
reporterPedelacq et al. 2006

Output & readout

Type
fluorescent
Reporter
sfGFP
Readout
Fluorescence (flow cytometry on recovered cells)
Positive result
Signal reflects luminal choline load.

Performance

Limit of detection
BetI Marionette sensor: µM-mM choline (module-validated).
Dynamic range
~10 µM - 1 mM choline
Response time
~240 min
Device validated
No — design template (parts validated individually)

BetI is a characterised orthogonal Marionette sensor; integrated CRISPRi device is a design template. Relevant to TMAO/cardiovascular research.

Safety

Biosafety level
BSL-1 (non-pathogenic chassis)
GRAS chassis
No
Biocontainment
Probiotic E. coli Nissle host; add thyA/dapA auxotrophy for gut-restricted containment.
Field-deployable
Lab / supervised use

Probiotic chassis with a human-safety record; research / supervised clinical use only.

Build & run

#StageStep
1designDesign anti-reporter sgRNA
Target the reporter promoter; check Nissle off-targets.
2assemblyAssemble units
TU1: BetI + Pbet -> sgRNA. TU2: dCas9 + constitutive sfGFP. Low-copy vector.
3transformationTransform E. coli Nissle 1917
Select; add auxotrophic containment.
4inductionValidate in vitro
Confirm choline response across a standard curve before any animal work.
5readoutRecover and measure
Recover cells from stool; quantify fluorescence.

Source & parts

Design
Design template combining the Marionette BetI choline sensor with a dCas9 CRISPRi circuit in E. coli Nissle
Parts validated in
  • Meyer et al. 2019, Nat. Chem. Biol. (Marionette sensors, BetI)
  • Qi et al. 2013, Cell (CRISPRi)
License
Parts per their original sources; design template CC BY 4.0